Indentation of a layer on an elastic substrate: influence of thickness and elastic modulus of the coating

Authors

DOI:

https://doi.org/10.7242/1999-6691/2025.18.1.5

Keywords:

indentation, homogeneous and layered material, layer on a nonlinear-elastic substrate, indenter shape, contact area, computational and field experiments

Abstract

The indentation experiment consists in pressing a probe into the surface of a material. The study of the force response of the material depending on the displacement of the indenter (depth of indentation) allows the evaluation of surface mechanical properties. In the case of indentation of inhomogeneous (coated) hyperelastic materials, questions arise about the contact area required for calculating mechanical properties, as well as about the applicability of contact models developed for homogeneous linear-elastic materials. The shape of the indenter in the vicinity of the tip begins to play a role when indenting to a shallow depth and/or studying thin films (the real geometry of the tip). In this work, the finite-element method was used to analyze the indentation of a layer on a hyperelastic substrate by an indenter in the form of a truncated cone or a paraboloid of revolution. In this work, the finite element method was used to analyze the pressing of an indenter in the form of a truncated cone or a revolution paraboloid into the system of layer on a hyperelastic substrate. The size of the tip radius of the indenter, the elastic modulus of the layer and its thickness were varied. The dependences of the force response on the depth of indentation, the size of the contact area and the depth of penetration were obtained. It is shown that, when indenting the layer on a substrate, the contact depth differs significantly from that of a homogeneous material and is a function of the depth of indentation and the parameters of both the indenter and the surface of the system. Analytical approximations of the contact depth for the truncated conical indenter were obtained. The applicability of Sneddon’s equation (indentation of a homogeneous linear-elastic material) for the layer on a hyperelastic substrate was considered. The limitations on its use imposed indenter and material parameters were determined. It is shown that, if the indentation depth is of the order of the tip radius, simple expressions describing the indentation by a cylinder or a paraboloid without taking into account the real contact area can be used to estimate elastic modulus. Recommendations are given on the practical use of the obtained results, in particular, in the treatment of atomic force microscopy data.

Downloads

Download data is not yet available.
Supporting Agencies
The study was carried out with financial support from the Russian Science Foundation (project No. 23-22-00064).

References

Golovin Y.I. Nanoindentation and Mechanical Properties of Materials at Submicro- and Nanoscale Levels: Recent Results and Achievements. Physics of the Solid State. 2021. Vol. 63. P. 1–41. DOI: 10.1134/S1063783421010108

Morozov I.A., Uzhegova N.I. Determination of mechanical properties of materials in terms of models of interaction between AFM probe and sample surface. Computational Continuum Mechanics. 2014. Vol. 7, no. 4. P. 385–397. DOI: 10.7242/1999-6691/2014.7.4.37

Uzhegova N.I., Svistkov A.L. Multilevel analysis of the relief of a surface sample obtained by atomic force microscopy techniques. Computational Continuum Mechanics. 2016. Vol. 9, no. 3. P. 366–374. DOI: 10.7242/1999-6691/2016.9.3.30

Hertz H. Ueber die Berührung fester elastischer Körper.. Journal Für die Reine und Angewandte Mathematik. 1882b. Vol. 92. P. 156–171. DOI: 10.1515/crll.1882.92.156

Sneddon I.N. The relation between load and penetration in the axisymmetric boussinesq problem for a punch of arbitrary profile. International Journal of Engineering Science. 1965b. Vol. 3. P. 47–57. DOI: 10.1016/0020-7225(65)90019-4

Giannakopoulos A.E., Triantafyllou A. Spherical indentation of incompressible rubber-like materials. Journal of the Mechanics and Physics of Solids. 2007b. Vol. 55. P. 1196–1211. DOI: 10.1016/j.jmps.2006.11.010

Zhang M.- G., Cao Y.-P., Li G.-Y., Feng X.-Q. Spherical indentation method for determining the constitutive parameters of hyperelastic soft materials. Biomechanics and Modeling in Mechanobiology. 2014b. Vol. 13. P. 1–11. DOI: 10.1007/s10237-013-0481-4

Zhang Q., Li X., Yang Q. Extracting the isotropic uniaxial stress-strain relationship of hyperelastic soft materials based on new nonlinear indentation strain and stress measure. AIP Advances. 2018b. Vol. 8, no. 11. 115013. DOI: 10.1063/1.5063384

Kramer D., Huang H., Kriese M., Robach J., Nelson J., Wright A., Bahr D., Gerberich W.W. Yield strength predictions from the plastic zone around nanocontacts. Acta Materialia. 1998b. Vol. 47. P. 333–343. DOI: 10.1016/S1359-6454(98)00301-2

Mesarovic S.D., Fleck N.A. Spherical indentation of elastic–plastic solids. Proceedings of the Royal Society of London. Series A: Mathematical, Physical and Engineering Sciences. 1999b. Vol. 455. P. 2707–2728. DOI: 10.1098/rspa.1999.0423

Abetkovskaia S.O., Chizhik S.A., Rudnitsky V.A., Kren A.P. Evaluation of viscoelastic properties of materials by nanoindentation. Journal of Friction and Wear. 2010. Vol. 31. P. 180–183. DOI: 10.3103/S1068366610030049

Moreno-Flores S., Benitez R., Vivanco M.d., Toca-Herrera J.L. Stress relaxation microscopy: Imaging local stress in cells. Journal of Biomechanics. 2010b. Vol. 43. P. 349–354. DOI: 10.1016/j.jbiomech.2009.07.037

Chyasnavichyus M., Young S.L., Tsukruk V.V. Probing of Polymer Surfaces in the Viscoelastic Regime. Langmuir. 2014b. Vol. 30. P. 10566–10582. DOI: 10.1021/la404925h

Jafarbeglou F., Nazari M.A., Keikha F., Amanpour S., Azadi M. Visco-hyperelastic characterization of the mechanical properties of human fallopian tube tissue using atomic force microscopy. Materialia. 2021b. Vol. 16. 101074. DOI: 10.1016/j.mtla.2021.101074

Chen X., Vlassak J.J. Numerical study on the measurement of thin film mechanical properties by means of nanoindentation. Journal of Materials Research. 2001b. Vol. 16. P. 2974–2982. DOI: 10.1557/JMR.2001.0408

Bec S., Tonck A., Loubet J.L. A simple guide to determine elastic properties of films on substrate from nanoindentation experiments. Philosophical Magazine. 2006b. Vol. 86. P. 5347–5358. DOI: 10.1080/14786430600660856

Ogar P.M., Gorokhov D.B., Kozevnikov A.S. Effective elastic modulus of a layered body. Modern Technologies. System Analysis. Modeling. 2016. No. 4. P. 37–42.

Volkov S.S. Analytical solution to contact problem on spherical indenter penetration into soft elastic layer. Vestnik of Don State Technical University. 2012. Vol. 12, no. 7. P. 5–10.

Useinov A.S., Radzinsky S.A., Kravchuk K.S., Zolkina I.Y., Andreeva T.I., Simonov-Emelyanov I.D. Physical and mechanical properties of siloxane coating on polymer substrates. Plasticheskie Massy. 2012. No. 4. P. 14–24.

Hasan M.M., Johnson C.L., Dunn A.C. Soft Contact Mechanics with Gradient-Stiffness Surfaces. Langmuir. 2022b. Vol. 38. P. 9454–9465. DOI: 10.1021/acs.langmuir.2c00296

Bahr D.F., Woodcock C.L., Pang M., Weaver K.D., Moody N.R. Indentation induced film fracture in hard film – soft substrate systems. International Journal of Fracture. 2003b. Vol. 119/120. P. 339–349. DOI: 10.1023/A:1024979030155

Zha X., Jiang F., Xu X. Investigation of modelling and stress distribution of a coating/substrate system after an indentation test. International Journal of Mechanical Sciences. 2017b. Vol. 134. P. 1–14. DOI: 10.1016/j.ijmecsci.2017.10.002

Morozov I.A., Beliaev A.Y., Kamenetskikh A.S. Strain-Induced Damageability of Elastic-Plastic Carbon Nanocoatings on a Polymer Substrate. Russian Physics Journal. 2023b. Vol. 66. P. 852–859. DOI: 10.1007/s11182-023-03014-y

Oliver W.C., Pharr G.M. Measurement of hardness and elastic modulus by instrumented indentation: Advances in understanding and refinements to methodology. Journal of Materials Research. 2004b. Vol. 19. P. 3–20. DOI: 10.1557/jmr.2004.19.1.3

Zhang Y., Wang H., Li X., Tang H., Polycarpou A.A. A finite element correction method for sub-20 nm nanoindentation considering tip bluntness. International Journal of Solids and Structures. 2017b. Vol. 129. P. 49–60. DOI: 10.1016/j.ijsolstr.2017.09.015

Owen D.S. Toward a better modulus at shallow indentations–Enhanced tip and sample characterization for quantitative atomic force microscopy. Microscopy Research and Technique. 2023b. Vol. 86. P. 84–96. DOI: 10.1002/jemt.24261

Yu N., Polycarpou A.A., Conry T.F. Tip-radius effect in finite element modeling of sub-50 nm shallow nanoindentation. Thin Solid Films. 2004b. Vol. 450. P. 295–303. DOI: 10.1016/j.tsf.2003.10.033

Smirnov S.V., Ekzempliarova E.O. Effect of the indenter tip radius on the stress-strain state of elastoplastic materials. Physical Mesomechanics. 2009. Vol. 12, no. 6. P. 73–78.

Morozov I.A., Izyumov R.I. Challenges of reliable AFM-tip shape reconstruction and approximation. Microscopy Research and Technique. 2024b. Vol. 87. P. 105–113. DOI: 10.1002/jemt.24415

Nguyen Q.D., Chung K.-H. Effect of tip shape on nanomechanical properties measurements using AFM. Ultramicroscopy. 2019b. Vol. 202. P. 1–9. DOI: 10.1016/j.ultramic.2019.03.012

Pharr G.M., Oliver W.C., Brotzen F.R. On the generality of the relationship among contact stiffness, contact area, and elastic modulus during indentation. Journal of Materials Research. 1992b. Vol. 7. P. 613–617. DOI: 10.1557/JMR.1992.0613

Saha R., Nix W.D. Effects of the substrate on the determination of thin film mechanical properties by nanoindentation. Acta Materialia. 2002b. Vol. 50. P. 23–38. DOI: 10.1016/S1359-6454(01)00328-7

Hay J.C., Bolshakov A., Pharr G.M. A critical examination of the fundamental relations used in the analysis of nanoindentation data. Journal of Materials Research. 1999b. Vol. 14. P. 2296–2305. DOI: 10.1557/JMR.1999.0306

Chung J.Y., Nolte A.J., Stafford C.M. Surface Wrinkling: A Versatile Platform for Measuring Thin-Film Properties. Advanced Materials. 2011b. Vol. 23. P. 349–368. DOI: 10.1002/adma.201001759

Chudinov V.S., Shardakov I.N., Ivanov Y.N., Morozov I.A., Belyaev A.Y. Elastic Modulus of a Carbonized Layer on Polyurethane Treated by Ion-Plasma. Polymers. 2023b. Vol. 15, no. 6. 1442. DOI: 10.3390/polym15061442

Published

2025-04-17

Issue

Section

Articles

How to Cite

Morozov, I. A., Beliaev, A. Y., & Izumov, R. I. (2025). Indentation of a layer on an elastic substrate: influence of thickness and elastic modulus of the coating. Computational Continuum Mechanics, 18(1), 57-67. https://doi.org/10.7242/1999-6691/2025.18.1.5